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Please use this identifier to cite or link to this item: http://hdl.handle.net/10553/74777
DC FieldValueLanguage
dc.contributor.authorZubar, Viktoriiaen_US
dc.contributor.authorLebedev, Yuryen_US
dc.contributor.authorAzofra Mesa, Luis Miguelen_US
dc.contributor.authorCavallo, Luigien_US
dc.contributor.authorEl-Sepelgy, Osamaen_US
dc.contributor.authorRueping, Magnusen_US
dc.date.accessioned2020-10-15T13:29:23Z-
dc.date.available2020-10-15T13:29:23Z-
dc.date.issued2018en_US
dc.identifier.issn1433-7851en_US
dc.identifier.urihttp://hdl.handle.net/10553/74777-
dc.description.abstractThe first base-metal-catalysed hydrogenation ofCO2-derived carbonates to alcohols is presented. The reactionproceedsundermildconditionsinthepresenceofawell-defined manganese complex with aloading as lowas0.25 mol%. The non-precious-metal homogenous catalyticsystem provides an indirect route for the conversion of CO2into methanol with the co-production of value-added (vicinal)diols in yields of up to 99%. Experimental and computationalstudies indicate ametal–ligand cooperative catalysis mechanism.en_US
dc.languageengen_US
dc.relation.ispartofAngewandte Chemie - International Editionen_US
dc.sourceAngewandte Chemie - International Edition [ISSN 1433-7851], v. 57, p. 13439 –13443en_US
dc.subject221001 Catálisisen_US
dc.titleHydrogenation of CO2-Derived Carbonates and Polycarbonates to Methanol and Diols by Metal-Ligand Cooperative Manganese Catalysisen_US
dc.typeinfo:eu-repo/semantics/articleen_US
dc.typeArticleen_US
dc.identifier.doi10.1002/anie.201805630en_US
dc.description.lastpage13443en_US
dc.identifier.issue41-
dc.description.firstpage13439en_US
dc.relation.volume57en_US
dc.investigacionCienciasen_US
dc.type2Artículoen_US
dc.description.numberofpages5en_US
dc.utils.revisionSíen_US
dc.identifier.ulpgcNoen_US
dc.description.sjr5,478
dc.description.jcr12,257
dc.description.sjrqQ1
dc.description.jcrqQ1
dc.description.scieSCIE
item.fulltextCon texto completo-
item.grantfulltextopen-
crisitem.author.deptGIR IUNAT: Fotocatálisis y espectroscopía para aplicaciones medioambientales.-
crisitem.author.deptIU de Estudios Ambientales y Recursos Naturales-
crisitem.author.orcid0000-0003-4974-1670-
crisitem.author.parentorgIU de Estudios Ambientales y Recursos Naturales-
crisitem.author.fullNameAzofra Mesa, Luis Miguel-
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