Identificador persistente para citar o vincular este elemento: http://hdl.handle.net/10553/122807
Título: Sustainable Nitrogen Activation – Are We There Yet?
Autores/as: MacFarlane, Doug
Simonov, Alexandr N
Vu, Th
Johnston, Sam
Azofra Mesa, Luis Miguel 
Clasificación UNESCO: 230320 Compuestos del nitrógeno
250105 Química atmosférica
Fecha de publicación: 2023
Publicación seriada: Faraday Discussions 
Resumen: The activation of dinitrogen as a fundamental step in reactions to produce nitrogen compounds, including ammonia and nitrates, has a cornerstone role in chemistry. Bringing together research from disparate fields where this can be achieved sustainably, this Faraday Discussion seeks to build connections between approaches that can stimulate further advances. In this paper we set out to provide an overview of these different approaches and their commonalities. We explore experimental aspects including the positive role of increasing nitrogen pressure in some fields, as well as offering perspectives on when 15N2 experiments might, and might not, be necessary. Deconstructing the nitrogen reduction reaction, we attempt to provide a common framework of energetic scales within which all of the different approaches and their components can be understood. On sustainability, we argue that although green ammonia produced from a green-H2 fed Haber-Bosch process seems to fit the bill, their remain many real-world contexts in which other, sustainable, approaches to this vital reaction are urgently needed
URI: http://hdl.handle.net/10553/122807
ISSN: 1359-6640
DOI: 10.1039/D3FD00087G
Fuente: Faraday Discussions [ISSN 1359-6640], 2023
Colección:Artículos
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